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Modern Optics

and Photonics of Nano- and Microsystems

Modern Optics and Photonics of Nano- and

Microsystems

CRC Press

Taylor & Francis Group

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1.

1.1.

1.2.

1.3.

1.3.1.

1.3.2.

1.3.3.

1.4.

2.

3.3.

3.3.1.

3.3.2.

4.3. Ph ase self-modulation of radiation in optical fibres 110

4.4. E ffect of dispersion on nonlinear processes in optical fibres 114

4.5. Ph ase cross-modulation of pulses in fibre guides 117

4.6. Fo ur-wave mixing of waves 119

4.7. St imulated Raman scattering (SRS) radiation in optical f ibres 122

4.8. St imulated Mandel’shtam–Brillouin scattering in optical f ibres 1

4.9. The propagation of ultrashort laser pulses in optical fibres

4.9.1. Pumping in the region of normal dispersion

4.9.2. Pumping in the region of anomalous dispersion

4.10. Ge neration of a supercontinuum in optical fibres 141

4.11. No nlinear properties of photonic crystal fibres 1 43

4.11.1. Dispersive properties of microstructured (MS) optical fibres

4.11.2. Generation of a supercontinuum in MS optical fibres, f or which the pump pulse wavelength lies in the region of a nomalous dispersion

4.11.3. Generation of supercontinuum in MS fibre lightguides in p umping in the region of normal dispersion 164

4.11.4. Generation of supercontinuum in MS optical fibres having t wo zero-dispersion wavelengths 167

4.11.5. Nonlinear optical properties of holey PC optical fibres 173

5.1. T he principle of

5.1.1.

5.1.2. Resonators of fibre lasers

5.1.2.1. Fabry–Perot type resonators

5.1.2.2. Ring fibre resonators

5.1.2.3. Resonator based on fibre Bragg gratings

5.1.3. Special features of active lightguides as a medium of a mplification of radiation 194

5.2. C ontinuous fibre lasers

5.2.1. Fibre lasers based on active fibres doped with neodymium (Nd 3+)

5.2.2. Lasers based on active lightguides of doped with ytterbium (Yb3 +) 198

5.2.3. Fibre-based lasers based on active optical fibres doped with e rbium ions (Er 3 + ). 199

5.2.4. Fibre lasers based on active optic fibres, doped with thulium ions (Tm 3+). 201

5.2.5. Fibre-based lasers based on active optical fibres, doped with h olmium ions (Ho 3+ ) 202

5.3. Fi bre lasers based on stimulated Raman scattering of radiation ( fibre SRS lasers) 2 03

5.3.1. The phenomenon of stimulated Raman scattering of ra diation in optical fibres

5.3.2. Fibre-optic SRS lasers

5.3.2.1. Single-stage SRS lasers

5.3.2.2. Multistage SRS lasers

5.3.2.3. Composite SRS lasers

5.3.2.4. Fibre-optic SRS lasers with random distributed feedback

5.4. Pu lsed fibre lasers 2

5.4.1. Methods for obtaining pulsed radiation from fibre lasers

5.4.1.1. Modulation of the quality factor of fibre lasers 219

5.4.1.2. Generation of pulsed radiation due to mode-locking

5.4.2. Compensation of dispersion spreading pulses

5.4.2.1. Prism compensators of group velocity dispersion 247

5.4.2.2. Grating compensator of the group velocity dispersion 2 50

5.4.2.3. Compensator for group velocity dispersion based on the Gi res–Tournois interferometer

5.4.2.4. Compensators of group velocity dispersion based on chirped B ragg mirrors

5.4.3. Amplification of ultrashort

6.

6.1. Mo rphology and physico-chemical characteristics of sp icules of deep-sea glass sponges 2 69

6.2. T he role of the photonic-crystal properties of the spicules o f deep-sea sponges during their metabolism 2 77

6.3. No nlinear optical properties of the spicules of deep-sea g lass sponges 2 80

6.4. B iomimetic modelling of biosilicate nanocomposite m aterial of DSGS spicules 283

6.4.1. Sol-gel technology of chemical modelling of biomineral ma terials and their optical characteristics 283

6.4.2. 2-D and 3-D biomimetic nanocomposite biomineral st ructures for photonics, biomedicine, catalysis and sorption 286

6.5. B iosilification in living systems using cloned proteins silicateins 2 91

7. Dynamic Holography and Optical Novelty-Filters

7.1. T he interaction of two plane waves on dynamic holograms i n photorefractive crystals 2 98

7.2. T he transfer characteristic of an optical Novelty-filter 3 02

7.3. Fe atures of optical Novelty-filters 3 06

7.3.1.

7.4.

7.4.1.

7.4.2.

8.2.

8.3.

8.3.1.

8.3.2.

9.5.1.

9.6.

9.6.1.

9.6.2.

10.1.1.1. Energy spectrum of charge carriers in the bulk crystal structure 397

10.1.1.2. Density of electron states in the energy band 398

10.1.2. One-dimensional isolated quantum well and quantum thread 399

10.1.2.1. One-dimensional isolated quantum well 400

10.1.2.2. Quantum thread 4 03

10.1.2.3. The density of electron states for an isolated onedimensional quantum well 4 05

10.1.2.4. The density of states for a quantum thread 4 07

10.1.3. Quantum dots and the density of states of electrons in them 408

10.2. Exciton states in semiconductor and dielectric materials 411

10.2.1. Free excitons or Wannier–Mott excitons 411

10.2.2. Bound excitons (Frenkel excitons) 418

10.3. Influence of the form of nanoparticles on the energy subsystem of charge carriers 4 20

10.3.1. Single-particle states in the nanoparticles of the complicated shape 422

10.3.2. Two-particle (exciton) states in nanoparticles with irregular shape geometry 426

10.4. Influence of the environment on the energy spectrum of excitons in nanoparticles 432

10.5. Low-energy optical nonlinearity of liquid nanocomposite media based on nanoparticles 4 44 Index

Introduction

Three decades, covering the end of the XX century and the beginning of the XXI century, are characterized by rapid progress in the development and implementation of technologies based on the achievements of photonics. Photonics is an interdisciplinary scientific field, which is based on fundamental and applied research related to the study of the properties of optical radiation, processes and technologies of generation and control of light characteristics, the phenomena of interaction of radiation with the matter, the processes of transmission and processing of optical signals, fib re optic communication and development of complex information systems.

Optical sciences, which are one of the earliest and most important areas of research in the field of physical sciences, are now actively penetrating into diverse fields of research, including chemistry, biology, medicine and engineering. In this regard, the world trends in the development of optics, optical instrumentation and optical material science have undergone significant changes in recent years. The changes touched upon the development of a new generation of optical materials, the discovery of new optical phenomena and effects, which formed the basis for the creation of fundamentally new optical elements, devices and systems. Today, photonics is seen as a priority direction for the development of science and technology in many leading countries of the world, as it serves as a key element for solving many social problems: from energy generation and its effective use, to ensuring public health, security, adequate response to climate change, etc.

Considering the foregoing, modern ideas about the development of optics and photonics, as fundamental foundations for the development of scientific and industrial

instrument making in the ranges of X-ray, ultraviolet, visible, infrared and terahertz electromagnetic radiation, do not allow a contrast boundary between them.

The experimental and theoretical results achieved in optics and photonics allowed us to develop new technologies that significantly transformed our life. First of all, it concerns the rapid development of communication systems and information technologies, as well as the implementation of laser technologies in industry and medicine. The number of new scientific results obtained in the field of optics and photonics is rapidly growing. Only since the 80-ies of the last century seven Nobel Prizes in Physics were received for the research performed in these areas. In this connection, it is extremely difficult to state all the results achieved in one monograph. This monograph is devoted to several key achievements of modern photonics and optics, which are presented in the following 10 chapters:

1. Fundamentals of nonlinear optics;

2. Phenomena of filamentation and generation of a supercontinuum in the propagation of laser pulses in a nonlinear medium;

3. Photonic crystals;

4. Nonlinear optics of optical fib re s;

5. Fib re lasers;

6. Photonics of self-organizing nanostructured biomineral objects and their biomimetic analogs;

7. Dynamic holography and optical Novelty filters;

8. Adaptive optoelectronic systems SMART-GRID monitoring of physical fields and objects;

9. Laser cooling, trapping and controlling atoms;

10. Photonics of nanostructures.

The material of these chapters is devoted to the consideration of the processes of linear and nonlinear propagation of laser pulses in volume and light-guiding media, new sources of coherent radiation-fib re lasers, photonic crystal objects created by living Nature, and new photonic information systems using dynamic spatial filters and distributed fib re -optic measurement systems, as well as achievements in the field of ultra-low laser cooling of atoms and studies of the optical and nonlinear optical properties of heterogeneous nanostructured systems .

The content and construction of the monograph are very close to the corresponding course “Modern optics”, which the author has read over the past two years to graduate and postgraduate students of the National Research Nuclear University “MEPhI” and the Institute of Automation and Control Processes, Far Eastern Branch of the Russian Academy of Sciences.

Since a significant part of the material presented in the monograph has not yet been reflected in the curriculum literature and remains to be described only in original articles and monographs, the author hopes that this monograph will be useful both to specialists and students and graduate students making their first steps in such fascinating areas of research which are modern optics and photonics.

Fundamentals of Nonlinear Optics

Introduction

When in ordinary life we talk about the propagation of light in matter, it is initially assumed that the characteristics of the medium do not change under its influence. Indeed, the electric fields in atoms and molecules, which are the main elements determining the structure and optical properties of matter, are very large. In this connection, the light sources that existed in the pre-laser era could provide electric fields in the light electromagnetic wave many orders of magnitude smaller than the intra-atomic ones. Therefore, the influence of the electromagnetic field of the lightwave on the properties of the medium turned out to be negligibly small and did not manifest itself under real conditions. Since in this case the response of the medium to the external optical action is proportional to the electric field strength in the wave, the theoretical description of the phenomena arising in the interaction of light with matter is usually called linear optics.

The discovery of optical quantum generators (lasers) made it possible to generate optical fields with a strength comparable to that of an intra-atomic field. The effect of such optical radiation on the medium leads to a change in its optical properties. This means that the wave in the medium experiences both self-action and can influence the propagation of other waves in the medium. Naturally, this leads to the emergence of new phenomena that have not been observed before and requires the development of new theoretical approaches. As a result, a new field of science arose, which was called the nonlinear optics.

The term ‘nonlinear optics’ was first introduced by the Russian scientist S.I. Vavilov in 1925, who managed to observe a decrease

in the absorption of light by uranium glasses when optical radiation passes through them with high intensity. In the early 60s of the same century, after the creation of lasers, nonlinear optical phenomena became not only observable, but also turned into a serious tool for studying matter, and became the basis for the creation of completely new laser devices. Thus, the subject of nonlinear optics are the processes of interaction of light with matter, the nature of which depends on its intensity. Such processes include phenomena of resonant medium clarification, two-photon or multiphoton light absorption, optical breakdown of the medium, generation of optical harmonics, ‘straightening’ of light, stimulated light scattering, selffocusing of light beams, self-modulation of pulses, and a number of other effects manifested in fields of laser radiation. The classification of all these nonlinear optical effects is presented in detail in [ 1 – 5 ].

Incoherent nonlinear optical effects . Such optical characteristics of the medium, as the refractive index and the absorption coefficient, do not depend on the intensity of light if the reaction of the medium to the electric field of the lightwave is described by linear material equations. In a constant or slowly varying external electric field with a sufficiently low value of the field strength, the polarization vector of the medium P , as a rule, depends linearly on the field strength vector E of the lightwave and is described by the following material equation [ 6 ]:

the CGS system

the International System of Units system

where ε 0 is the dielectric constant. ( Further, the formulas in this chapter are given only in the CGS system in which ε 0 = 1).

The proportionality coefficient χ is called the dielectric susceptibility or the polarizability of the medium and depends on the properties of the medium: chemical composition, concentration, structure, aggregate state of the medium, and also on temperature, mechanical stress, etc.

However, this material equation is approximate since it is valid only for the electric field of the lightwave E small compared with the intensity of intra-atomic electric fields E a . To estimate the value of E a we can assume that the order of magnitude is E a ~ e / a 2 , where a is the size of the atom, e is the electron charge. As a ~ 10 −8 cm, then the intra-atomic electric field will be of the order of E a ~ 10 8 V/cm.

In light beams from non-laser sources, the field strengths do not exceed 0.1−10 V/cm and the linear material equations ( 1.1 ), ( 1. 2) are satisfied with great accuracy. However, in intense laser beams, the field strength E reaches values of 10 6 −10 7 V/cm. In such fields, the model of a harmonic oscillator for describing the behaviour of an optical electron in an atom is no longer applicable and the relationship between the polarizability of the medium and the intensity of the light-wave field becomes nonlinear. As a result, the optical characteristics of the medium depend on the radiation intensity, which does not lead to any small corrections, but to fundamentally new effects that are not observed in linear optics.

Nonlinear optics significantly expands our understanding of the interaction of light with matter. For example, in the earliest experiments on nonlinear optics carried out by S.I. Vavilov and V.L. Levshin, a slight decrease (up to 1.5%) of the uranium glass absorption coefficient with increasing light intensity was observed. The appearance of this nonlinear saturation effect is due to the alignment of populations of two energy levels between which quantum transitions occur with the absorption and emission of light. Subsequently, the decrease in the fraction of the absorbed power with increasing light intensity, that is, the clarification??? of the nonlinear absorbing medium during passage of strong light beams, has found application in laser technology where it is used to modulate the quality of optical resonators for the purpose of generating ultrashort high-power pulses (see, for example, Chapter 5 ). In this case, a cell with a nonlinear absorbing medium is an automatic shutter opening under the influence of a powerful light beam. It is very important that such a shutter has a low inertia, since after passing a powerful light pulse, the medium quickly becomes again opaque for the low-intensity light. In an active medium with population inversion, the saturation effect leads to a decrease in the gain with increasing light intensity and, thus, to the establishment of a steady-state lasing regime in lasers. If the medium is opaque for the low-intensity light due to the saturation effect becomes transparent in strong light fields, then the opposite situation is observed in the

optical transparency region of the medium. Here, as a result of multiphoton absorption of radiation, intense light can be absorbed much more strongly than weak light. At high radiation densities, a system with energy levels E 1 and E 2 can absorb in an elementary act two photons with frequencies ω 1 and ω 2 , such that ħω 1 + ħω 2 = E 2 − E 1. In particular, in the first case, when ω 1 = ω 2 = ( E 2 − E 1)/2 ħ , the probability of absorption of two photons is proportional to the product of the intensities of the beams with frequencies ω 1 and ω 2 (or the square of their intensity for ω 1 = ω 2 ).

Nonlinear incoherent effects include the multiphoton process of radiation absorption. For example, in the act of interaction of light with the medium, it is possible to simultaneously absorb three photons or more. Multiphoton absorption is used in nonlinear laser spectroscopy and allows obtaining information on the energy levels of quantum systems.

In experiments with focused laser beams, such high light-field intensities are attained when the processes in which the atom absorbs eight or more photons become available to observation. As a result, photoionization of the atom with he light of low frequency can occur, that is, in the intense light fields, the red boundary of the photoelectric effect disappears.

One of the most striking examples of nonlinear incoherent effects is the self-focusing of light. The effect is that the medium acquires focusing (lens) properties in the field of a powerful laser beam. As a result, the light beam ‘collapses’, turning into a thin luminous filament, or breaks up into several such filaments (the phenomenon is considered in Chapter 2 ). The mechanism of self-focusing is associated with a change in the refractive index of the medium under the action of a powerful lightwave. The reasons for this may be different. For example, the electrostriction in a light field leads to the appearance of a pressure that changes the density of the medium in the region occupied by the light beam, and, consequently, also changes the refractive index of the medium. In a liquid, a strong light field leads to the orientation of anisotropically polarizable molecules due to the interaction of light with the induced dipole moment, while the medium becomes anisotropic, and the average refractive index for the orienting field increases. This effect is commonly called the high-frequency Kerr effect. The change in the refractive index here, as in the well-known static Kerr effect, is due to the ‘alignment’ of molecules over the field.

Finally, the change in the density, and, consequently, in the refractive index of the medium can be associated with heating caused by the dissipation of the energy of a powerful lightwave.

The self-focusing of light was theoretically predicted by G.A. Askar’yan in 1962, and experimentally first observed by N.P. Pilipetskii and A.R. Rustamov in 1965. In their experiments, narrow luminous filaments were photographed in organic liquids irradiated by a focused beam of a ruby laser.

The self-defocusing effect is inverse to self-focusing. Under the action of high-power laser radiation, a nonlinear addition to the absorption index appears in the medium. In the event that this additive is positive, self-focusing takes place (a nonlinear positive quasilens is formed). With a negative addition, the refractive index on the beam axis decreases and a nonlinear negative quasilens is formed, which leads to self-defocusing of the radiation. Thus, when laser radiation passes through a liquid, even its weak absorption leads to thermal expansion of the liquid, a decrease in its density, and, as a consequence, its refractive index. Ultimately, this leads to the formation of a thermal defocusing lens, which increases the angular divergence of the laser beam.

The same mechanisms cause another effect of nonlinear self-action of light – self-modulation of the light pulse. In self-modulation of a pulse, which, for example, can occur in an optical fibre, the frequency spectrum of the pulse drastically broadens, which makes it possible, by subsequent compression, to obtain extremely short light pulses. This effect is used in the systems of generation of femtosecond laser pulses.

We note that the main feature of the incoherent nonlinear optical effects considered above is their independence from the phase of laser radiation.

Nonlinear optical effects due to high coherence of radiation . It is known that in addition to high intensity, laser radiation has a high degree of coherence. The latter is manifested in nonlinear optical effects, in which the phase relations play a decisive role. Such effects include: harmonic generation, frequency mixing, stimulated Raman scattering of light, and violation of the superposition principle for strong lightwaves in a medium.

Generation of harmonics. Frequency mixing . This phenomenon, for example, consists in doubling the frequency of light in the propagation of a powerful laser beam in a crystal. The mechanism

of the process is related to the nonlinearity of an elementary atomic oscillator. The doubling of the frequency of light in the crystal was the first coherent nonlinear optical effect discovered shortly after the creation of the laser in 1961. In the experiments of the American scientist P. Franken, the radiation of a ruby laser having a wavelength of λ = 694.3 nm was focused into a quartz crystal. The radiation emerging from the crystal was unfolded into the spectrum with the aid of a dispersion prism and was focused on a photographic plate. Experience has shown that, in addition to the light at the frequency of the laser ( ω ), the light comes out of the crystal at a doubled frequency (the second harmonic) having a wavelength of λ 2 = λ/2 ( ω 2 = 2 ω ) = 347.15 nm. Despite the fact that the radiation second harmonic in P. Franken’s experiment was extremely weak, this experience played a fundamental role, initiating the development of nonlinear optics, and subsequent experiments showed that using other crystals, the efficiency of second harmonic generation can be dramatically increased. Methods for transforming a significant fraction of the laser radiation to the second harmonic have been developed; in some cases it is possible to obtain the lasing efficiency close to 100%.

In addition to generating the second harmonic, it is possible to generate total and difference radiation frequencies of two or more lasers: ω s = ω 1 ± ω 2 , as well as higher harmonics and total and difference frequencies in higher-order processes ω s = nω 1 ± mω 2 (where n and m are integers). Currently, this effect is widely used to convert the frequency of laser radiation and the development of spectral ranges in which the creation of lasers is difficult.

Stimulated Raman scattering of light . This effect (abbreviated SRS) consists in the fact that in the field of a powerful laser beam the medium generates intense radiation shifted in frequency relative to the laser by an amount equal to the frequency of molecular vibrations. The mechanism of the process is the same as in the case of spontaneous scattering – modulation of light by molecular vibrations. However, unlike spontaneous scattering, which is very weak and directed in all directions, stimulated scattering resembles laser generation. The power and directivity of the stimulated scattering are commensurable with the analogous parameters of the laser beam. The reason for this is that stimulated scattering does not occur on chaotic thermal molecular vibrations, but on vibrations excited and phased by light in a large volume of the medium. The transition of spontaneous scattering to stimulated scattering occurs

when the intensity of the exciting light exceeds a certain definite quantity called the SRS threshold.

For the first time stimulated Raman scattering was observed in 1962 by American scientists E. Woodbury and V. Nga in the study of the Q -switching regime of a ruby laser with the aid of a Kerr cell with nitrobenzene. They found the appearance of an infrared component in the laser radiation, the frequency of which was 1345 cm–1 lower than the frequency of the main laser radiation. Since the frequency shift coincided with one of the natural oscillation frequencies of the nitrobenzene molecule, it was suggested that the appearance of the infrared component is associated with the Raman scattering of light in nitrobenzene, and the high intensity of radiation is due to the forced character of the process, in which molecular vibrations are strongly swinging with light. This assumption was confirmed in subsequent experiments with various liquids, as well as with gases and solids. Experience shows that the stimulated Raman scattering is observed only at a sufficiently high light intensity achieved by focusing the beam into a cuvette. Since stimulated scattering has a high intensity, commensurate with the intensity of the laser beam, this circumstance makes it possible to create effective laser transducers radiation based on the SRS process. Currently, such converters are used to convert the radiation frequency, as well as to compress (shorten the duration and increase the power) of laser pulses. In addition, based on the SRS process, it is possible to carry out a coherent summation of the emissions of several laser modules. The excitation of coherent molecular vibrations with the aid of a pair of lightwaves (the method of biharmonic pumping) is also widely used in the spectroscopy of coherent anti- Stokes scattering of light (CARS).

Violation of the superposition principle for strong lightwaves in a medium. The principle of superposition is that different lightwaves, differing in frequency, direction of propagation or polarization, propagate and interact with the environment independently of each other. In nonlinear optics this is not so. As we have seen, new spectral components of the field appear in nonlinear optical processes, different lightwaves interact strongly with each other, energy is exchanged between them until the complete transformation of one wave into another. A typical example of this kind is the generation of a second optical harmonic. Thus, for nonlinear-optical processes of interaction of radiation with matter, a violation of the superposition principle is characteristic.

1.1. Polarization of dielectrics in a constant electric field

Any electromagnetic process in a medium is described by the Maxwell equations [ 6 ]

which in the operator form have the form

where E ( r , t ), H ( r , t ) are the vectors of electric and magnetic field strengths at a point with a radius vector r at the time t ; ρ is the density of electrical charges; j is the vector of current density; D and B are the vectors of electrical and magnetic inductions. However, these equations are not sufficient to solve the problem; we need material equations that establish additional connections between these vectors [ 2 – 6 ]:

We recall that in the International System of Units the equations ( 1.5 ) will have the form

where ε 0 and μ 0 are the dielectric and magnetic constants, ε and μ are the dielectric and magnetic permeabilities of the medium, and σ is the electric conductivity of the medium.

Equations ( 1.5 ) establish a connection between the vector of macroscopic polarization of the medium P , the vector of the macroscopic magnetization of the medium M and vectors D and B , as well as between the current density j and the electric field strength E . Further, we will not take into account the magnetic properties of the medium.

In the isotropic case, the macroscopic polarization of the medium depends on the electric field strength. The coefficient of proportionality in such a dependence is the dielectric susceptibility of the medium χ( E ), which in general also depends on E . If we take this dependence into account, then, using ( 1.1 ) and ( 1.5 ), we obtain:

The value ε ( E ) = 1+ χ ( E ) is called the dielectric permittivity of the medium.

In weak fields, the dielectric susceptibility of the medium and the permittivity are constants that do not depend on the electric field strength and, consequently, the reaction of the medium to the external field is linear:

Nonlinear effects are manifested only when the fields are strong enough and the quantities χ and ε can no longer be regarded as independent of the field strength. To illustrate the appearance of the nonlinear dependence of the quantities χ and ε , we calculate them in the framework of a simple classical problem. To do this, let us consider a gas consisting of the simplest atoms (two point charges of the quantity e : a nucleus and an electron) without a constant electric dipole moment. In the absence of an external field, the position of the mass centred for point charges in the atom is the same. If the atomic gas is placed in a constant electric field, then the charges in each atom will move a certain distance r . For simplicity, we assume that the electron displacement coincides with the direction of the

external electric field. Then we can ignore the vector nature of the quantities involved in the problem, and operate with scalar quantities. Thus, atoms will acquire a dipole moment: d = e ∙ r

If the environment consists of N atoms, then its macroscopic polarization will be

Two forces act on an electron in an atom: one acts on the side of the electric field with force F E = eE , and the second – elastic, due to the potential field in which the electron moves, returning the electron to its former position, with force: F el = − kr − qr 3 (this force in the general case depends nonlinearly on the electron displacement) [ 4 ], where k and q are the linear and nonlinear elastic deformation constants. Equating the forces F E and F y , we obtain an equation for determining the amount of displacement of an electron in an external field:

Determining the value r from (1.9) and substituting its value in (1.10), we obtain a nonlinear equation for the polarization of the medium:

We represent the polarization of the medium in the form P = P L + δ Р, where P L is a linear component of the polarization of the medium, independent of the magnitude of the electric field, and δP is a small nonlinear addition to polarization. We solve equation ( 1.11 ) with respect to P , assuming that the power term of P 3 is small. In this connection, equation ( 1.11 ) can be represented as a system of two equations: one for the terms of the zeroth and the other for the terms of the first order of smallness:

Using the system ( 1.12 ), we obtain an expression for the polarization of the medium:

Comparing the solution obtained with ( 1.7 ), we obtain

As can be seen, the dielectric susceptibility of the medium is a function of the electric field strength. If the magnitude of the field is sufficiently weak (much less than the intra-atomic field), then the second term in ( 1.14 ) can be neglected (this means that the displacement is small and in the expression for the term it can be neglected) and the dielectric susceptibility of the medium becomes a constant.

Before that, we considered the case of an isotropic medium. When the medium is anisotropic, the dielectric susceptibility and permeability of the medium, instead of scalars, become tensors of the second rank, and the connection between the vectors P , D , E has the form:

where d ij is the unit tensor, ε ij ( E ) ─ in the general case, the tensor of the permittivity of the medium, which depends on the magnitude of the electric field strength.

In the Cartesian coordinate system, the components of the vector D are represented as:

Using these relations, knowing the parameters of the external electric field and the dielectric susceptibility tensor of a particular anisotropic medium (usually determined by experimental methods), one can always calculate its polarization.

1.2. Polarization of an isotropic dielectric in a light field

Let us consider the polarization of a dielectric in a high-frequency light field using the same simple gas model. Since the intensity of the electric field now depends on time, it is necessary to solve the dynamic, and not static, problem for the motion of an electron. The equation of motion of the electron is written in the form

where F f is the friction force proportional to the velocity of motion of the electron, γ f is the coefficient of friction; F E is a force acting on the side of the external electric field; F ef is the elastic force. For the case of a weak electric field, we can use the first approximation for the elastic force: F ef = − kr. Substituting this expression in ( 1.18 ), we obtain

We multiply the last equation in ( 1.19 ) by eN , taking into account the expression for the polarization of the medium ( 1.9 ) and the expression for the natural frequency of the electron oscillations

ω 2 0 = k / m we obtain an equation for the polarization of the medium:

Fundamentals of Nonlinear Optics

If the lightwave changes in accordance with the harmonic law: E ( t ) = E 0 cos( ωt ), the solution for polarization will be found in the form P ( t ) = P 0 cos( ωt + φ ). Substituting this expression into ( 1.20 ) we obtain

(1.21)

Equating separately the terms at cos ωt and sin ωt , we obtain a system of equations

From the first equality, we determine the phase of the oscillations of polarization of the medium:

Using the second equality in ( 1.22 ) and the expression ( 1.23 ), we obtain the expression for the polarization amplitude of the medium:

As a result, the expression for the polarization of the medium has the following form

As indicated by the expression ( 1.25 ), the polarization of the

dielectric medium changes with the frequency of the light field wave ω and the polarization amplitude of the medium depends on the relationship between the intrinsic frequency of the oscillations of the electrons in the atom ω 0 and the frequency of the incident light radiation ω .

In most cases, some limiting cases are of special interest. In particular, when the frequency of the lightwave coincides with the intrinsic frequency of the oscillations of the electrons of the medium (resonance case): ω = ω 0, the polarization amplitude of the medium is maximum and equal to:

Another limiting case may be the large difference of the frequencies of the lightwave and the resonance frequency of the oscillations of the electrons of the medium: ω >> ω 0 or | ω – ω 0| >> γ T. Consequently, from ( 1.23 ) it follows that

This means that in this case the phase for the polarization of the medium is close to 0 and the polarization oscillations take place almost completely in the phase with the oscillations of the lightwave. Using equation ( 1.25 ), we derive the expression for the ionisation of the dielectric medium

As indicated by ( 1.28 ), the dielectric susceptibility of the medium depends on the frequency of light radiation.

Another limiting cases may be ω = 0 which indicates the effect of a direct electric field on the medium, consequently

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furnished, and then expressed his wish that upon his departure for the Northern frontier the whole wing, as the most separated, beautiful and desirable portion of the establishment, might be given up to the exclusive use of his affianced bride.

Mrs. Houston consented, with the proviso that he should not vacate the rooms until the hour of his departure for camp.

Accordingly, the first evening of Margaret’s arrival she had been accommodated with a pleasant chamber on the second-floor front of the main building.

But on Tuesday morning, after Mr. Helmstedt and Ralph Houston had departed, Mrs. Houston and her maids went busily to work and refreshed the two pretty rooms of the wing, hanging white lace curtains to the windows, white lace valances to the toilet table and tester, etc., and transfiguring the neatly-kept bachelor’s apartments into a lady’s charming little boudoir and bedchamber.

When all was arranged, even to the fresh flowers in the white vases upon the front room mantelpiece, and the choice books from Mrs. Houston’s own private library upon the center table, the busy little lady, in her eagerness to surprise and please, hurried away to seek Margaret and introduce her to her delightful apartments. She tripped swiftly and softly up the stairs, and into the room, where she surprised Margaret, quite absorbed in some work at her writing-desk.

“Oh, you are busy! Whom are you writing to, my dear?” she inquired eagerly, hastening to the side of the girl and looking over her shoulder

She meant nothing, or next to nothing—it was her heedless, impulsive way. She was in a hurry, and did not stop to remember that the question was rude, even when Margaret, with a sudden blush, reversed her sheet of paper, and, keeping her hand pressed down upon it, arose in agitation.

“Why, how startled you are, my dear! How nervous you must be! I ought not to have come upon you so suddenly. But to whom are you writing, my dear?”

“To—a—correspondent, Mrs. Houston.”

“Why, just look there now! See what a good hand I am at guessing, for I even judged as much! But who is your correspondent then, my dear?”

“A—friend! Mrs. Houston.”

“Good, again! I had imagined so, since you have no enemies, my child. But who then is this friend, you little rustic? You have not even acquaintances to write letters to, much less friends, unless it is Franky! Ah, by the way, don’t write to Franky, Margaret! He could not bear it now.”

Margaret made no comment, and Mrs. Houston, growing uneasy upon the subject of Franky, said:

“I hope you are not writing to Franky, Margaret!”

“No, Mrs. Houston, I am not.”

“If not to Franky, to whom then? It cannot be to your father or Ralph, for they have just left you. Come! this is getting interesting! Who is your correspondent, little one? Your old duenna insists upon knowing.”

Margaret turned pale, but remained silent.

“Dear me, how mysterious you are! My curiosity is growing irresistible! Who is it?”

Margaret suddenly burst into tears.

This brought the heedless little lady to her senses. She hastened to soothe and apologize.

“Why, Margaret, my dear child! Why, Margaret! Dear me, how sorry I am! I am very sorry, Margaret! What a thoughtless chatterbox I am of my age! But then I was only teazing you to rouse you a little, my dear! I did not mean to hurt you! And then I had such a pleasant surprise for you. Forgive me.”

Margaret slipped her left hand into Mrs. Houston’s (her right was still pressed upon the letter), and said:

“Forgive me. It is I who am nervous and irritable and require sufferance. You are very, very kind to me in all things, and I feel it.”

The little lady stooped and kissed her, saying:

“Such words are absurd between you and me, Maggie. Come, I will leave you now to finish your letter, and return to you by and by.”

And then she left the room, thinking within herself: “The sensitive little creature! Who would have thought my heedless words would have distressed her so? I did not care about knowing to whom the letter was written, I am sure. But, by the way, to whom could she have been writing? And, now I reflect, it was very strange that she should have been so exceedingly distressed by my questionings! It never occurred to me before, but it really was rather mysterious! I must try to find out what it all means! I ought to do so! I am her guardian, her mother-in-law. I am responsible for her to her father and to her betrothed husband.”

Meanwhile Margaret Helmstedt had started up, closed the door and turned the key, and clasping her pale face between her hands, began pacing the floor and exclaiming at intervals:

“Oh, Heaven of heavens, how nearly all had been lost! Oh, I am unfit, I am unfit for this dreadful trust! To think I should have set down to write to him, and left the door unfastened! Farewell to liberty and frankness! I am given over to bonds, to vigilance and secretiveness forever! Oh, mother! my mother! I will be true to you! Oh, our Father who art in heaven, help me to be firm and wise and true!”

She came back at last, and sat down to her writing-desk, and finished her letter. Then opening her pocketbook, she took out the check for five hundred dollars, drawn by her father, in her favor, on a Baltimore bank, inclosed it in the letter, sealed and directed it, and placed it in the sanctity of her bosom.

Then folding her arms upon her writing-desk, she dropped her head upon them, and in that attitude of dejection remained until the ringing of the supper bell aroused her.

Colonel Houston, who was waiting for her in the hall, received her with his old-school courtesy, drew her hand within his arm and led

her out upon the lawn, where, under the shade of a gigantic chestnut tree, the tea table was set—its snowy drapery and glistening service making a pleasant contrast to the vivid green verdure of the lawn upon which it stood. Old Colonel and Mrs. Compton and Nellie formed a pleasing group around the table. Colonel Houston handed Margaret to her place, and took his own seat.

“My dear, I am going to send Lemuel to Heathville to-morrow, and if you like to leave your letter with me, I will give it to him to put in the post office,” said Mrs. Houston.

“I thank you, Mrs. Houston,” said Margaret.

“Ah! that is what kept you in your room all the afternoon, my dear. You were writing a letter; whom were you writing to, my child?” said old Mrs. Compton.

“Pray excuse me,” said Margaret, embarrassed.

This answer surprised the family group, who had, however, the tact to withdraw their attention and change the subject.

After tea, an hour or two was spent upon the pleasant lawn, strolling through the groves, or down to the silvery beach, and watching the monotonous motion of the sea, the occasional leap and plunge of the fish, the solitary flight of a laggard water fowl, and perhaps the distant appearance of a sail.

At last, when the full moon was high in the heavens, the family returned to the house.

Mrs. Houston took Margaret’s arm, and saying:

“I have a little surprise for you, my love,” led her into the pretty wing appropriated to her.

The rooms were illumined by a shaded alabaster lamp that diffused a sort of tender moonlight tone over the bright carpet and chairs and sofa covers, and the marble-topped tables, and white lace window curtains of the boudoir, and fell softly upon the pure white draperies of the sleeping-room beyond.

Hildreth, in her neat, sober gown of gray stuff, and her apron, neckhandkerchief and turban of white linen, stood in attendance.

Margaret had not seen her faithful nurse for a month—that is, not since her mother’s decease—and now she sprang to greet her, scarcely able to refrain from bursting into tears. Mrs. Houston interfered.

“Now, my dear Margaret, here are your apartments—a sweet little boudoir and chamber, I flatter myself, as can be found in Maryland— connected with the house, yet entirely separate and private. And here are your servants; Hildreth will occupy the room in the roof above, and Forrest has a quarter in the grove there, within easy sound of your bell. Your boat is secure in the boathouse below, and your horse is in the best stall in the stable.”

“I thank you, dear Mrs. Houston.”

“I understand, also, that your father has assigned you a very liberal income. Consequently, my dear, you are in all things as independent as a little queen in her palace. Consider also, dear Margaret, that it is a great accession of happiness to us all to have you here, and we should wish to have as much of your company as possible. Therefore, when you are inclined to society, come among us; at all other times, you can retire to this, your castle. And at all times and seasons our house and servants are at your orders, Margaret; for you know that as the bride of our eldest son and heir, you are in some sort our Princess of Wales,” she concluded, playfully.

“I thank you, dear Mrs. Houston,” again said the young girl. Her thoughts were too gravely preoccupied to give much attention to the prattle of the lady.

“And by the way, Margaret, where is your letter, my dear? I shall dispatch Lemuel early in the morning.”

“You are very considerate, Mrs. Houston, but I do not purpose to send it by Lemuel.”

“As you please, my dear. Good-night,” she said, kissing the maiden with sincere affection, notwithstanding that, as she left the room, her

baffled curiosity induced her to murmur:

“There is some ill mystery, that I am constrained to discover, connected with that letter.”

Miss Helmstedt, left to herself, directed Hildreth to secure the doors communicating with the main building, and then go and call Forrest to her presence.

“I shall not tax you much, Forrest,” she said, “though to-night I have to require rather an arduous service of you.”

“Nothing is hard that I do for you, Miss Margaret,” replied Forrest.

“Listen then—to-night, after you are sure that all the family are retired, and there is no possibility of your being observed, take my horse from the stable, and ride, as for your life, to Belleview, and put this carefully in the post office,” she said, drawing the letter from her bosom and placing it in the hand of Forrest.

The old man looked at her wistfully, uneasily, drew a deep sigh, bowed reverently, put the letter in his pocket, and, at a sign from his mistress, left the room.

But that night at eleven o’clock, Nellie, watching from her window, saw Miss Helmstedt’s messenger ride away over the hills through the moonlight.

CHAPTER XI.

THE MYSTERIOUS CORRESPONDENT.

“You, sir! I want to see you! Come hither!” said Mrs. Houston, as she stood upon the back piazza, early the next morning, and beckoned Forrest to her presence.

The old man bowed in his deferential manner, advanced and stood hat in hand before the little lady.

“Where did you go last night after we had all retired?”

Forrest bowed again, humbly and deprecatingly, but remained silent.

“Did you hear me speak to you?” inquired Mrs. Houston, impatiently.

The old man bowed once more very meekly, and answered:

“I went after no harm, mistress.”

“Nor after any good, I’ll venture to say!—but that is not the point, sir. I ask you where you went! and I intend to have an answer.”

“I begs your pardon sincere, mistress, but mus’ ’cline for to ’form you.”

“You old villain! Do you dare to defy me here on my own premises?

I’ll see about this!” exclaimed the lady, in a voice more shrill than ladylike, as with a flushed face and excited air she turned into the house to summon Colonel Houston.

But she was intercepted by Margaret, who had heard the voice, and now came from her own apartment and stood before her.

“Stay, Mrs. Houston, I sent Forrest away on an errand, last night, and if he declined to inform you whither he went, it was from no disrespect to you; but from fidelity to me. I had enjoined him not to speak to any one of his errand,” she said, in a voice and manner so respectful as to take away everything offensive from her words.

“You did! Now then where did you send him, Margaret? I am your guardian, and I have a right to know.”

“You must forgive me, Mrs. Houston, if I decline to inform you,” replied the maiden, firmly, though still very respectfully.

“I know, however. It was to mail that letter.”

“You must draw your own conclusions, dear madam.”

“I know it was to mail that letter! And I will put on my bonnet and drive over to the post office, and demand of the postmaster to whom the letter mailed last night by the negro Forrest was directed! There’s not so many letters go to that little office but what he will be able to recollect!” exclaimed Mrs. Houston, angrily.

“Oh, God!”

The words breathed forth possessed so much of prayerful woe that the little lady half started, and turned back to see Margaret grow pale and sink upon the corner of the hall settee.

Mrs. Houston hesitated between her curiosity and anger on the one hand, and her pity on the other. Finally she made a compromise. Coming to Margaret’s side, she said:

“Maggie, I am treated abominably, standing as I do in your mother’s place toward you, and being as I am your guardian—abominably! Now I am sure I do not wish to pry into your correspondence, unless it is an improper one.”

“Mrs. Houston, my mother’s daughter could not have an improper correspondence, as you should be the first to feel assured.”

“Yet, Margaret, as it appears to me, if this correspondence were proper, you would not be so solicitous to conceal it from me.”

It occurred to Margaret to reply, “Mrs. Houston, suppose that I were writing sentimental letters to a female friend, which might not be really wrong, yet which I should not like to expose to your ridicule, would I not, in such a case, even though it were a proper correspondence, be solicitous to conceal it from you?”—but her exact truthfulness prevented her from putting this supposititious

case, and as she did not in any other manner reply, Mrs. Houston continued:

“So you see, Margaret, that you force me to investigate this matter, and I shall, therefore, immediately after breakfast, proceed to the village to make inquiries at the post office.” And having announced this resolution, the lady, still struggling with her feelings of displeasure, left the hall.

Margaret withdrew to her own sitting-room, and threw herself upon her knees to pray. Soon rising she touched the bell and summoned Forrest.

The old man came in looking very sorrowful.

“How did it become known that you left the premises last night, Forrest?”

“Somebody must o’ ’spicioned me, chile, an’ been on de watch.”

“Yes! yes! I see now! that was it; but, Forrest, this is what I called you to say: In future, whenever Mrs. Houston asks you a question about your services to your mistress, refer her to me.”

“Yes, Miss Marget.”

“You may go now.”

“Pardon, Miss Marget; I wants to say somefin as’ll set your min’ at ease ’bout dat letter.”

“Ah, yes, you mailed it?”

“True for you, Miss Marget; but listen; de pos’ office was shet up. So I jes drap de letter inter de letter-box. Same minit der was two colored boys an’ a white man drap as many as five or six letters in long o’ mine. So even ef de pos’masser could o’ see me t’rough de winder, which he couldn’t, how he gwine know which letter ’mong de half-dozen I drap in?”

“True! true! true! Oh, that was very providential! Oh, thank Heaven!” exclaimed Margaret, fervently clasping her hands. The old man bowed and retired.

After breakfast, Mrs. Houston, without explaining the motive of her journey to any one, ordered her carriage, and drove to the village as upon a shopping excursion.

Now you have not known Mrs. Nellie Houston thus long without discovering that with some good qualities, she was, in some respects, a very silly woman. She drove up to the post office, and by her indiscreet questions respecting “a certain letter mailed the night before by Forrest, the messenger of her ward, Miss Helmstedt,” set the weak-headed young postmaster to wondering, conjecturing and speculating. And when she found that he could give her no satisfaction in respect of the letter, she made matters worse by directing him to detain any letters sent there by her ward, Miss Helmstedt, unless such letters happened to be directed to a Helmstedt or a Houston, who were the only correspondents of Miss Helmstedt recognized by her family.

The postmaster thereupon informed Mrs. Houston, that if she wished to interfere with the correspondence of her ward, she must do so at her own discretion, and necessarily before they should be sent to his office, as he had no authority to detain letters sent thither to be mailed, and might even be subjected to prosecution for so doing.

Mrs. Houston went away baffled and angered, and also totally unconscious of the serious mischief she had set on foot.

To an idle and shallow young man she had spoken indiscreetly of the young maiden whose orphanage she had promised to cherish and defend, exposing her actions to suspicion and her character to speculation. She had left the spotless name of Margaret Helmstedt a theme of low village gossip.

And thus having done as much evil as any foolish woman could well do in an hour, she entered her carriage, and with the solemn conviction of having discharged her duty, drove home to the Bluff.

“God defend me, only, from my friends, for of my enemies I can myself take care,” prayed one who seemed to have known this world right well.

From that day Margaret Helmstedt, whenever she had occasion to write a letter, took care to turn the key of her room door; and whenever she had occasion to mail one, took equal precaution to give it, unperceived, into the hands of Forrest, with directions that he should drop it into the letter-box at a moment when he should see other letters, from other sources, going in. Poor girl! she was slowly acquiring an art hateful to her soul. And one also that did not avail her greatly. For notwithstanding all her precautions, the report crept about that Miss Helmstedt had a secret correspondent, very much disapproved of by her friends And in course of time also, the name of this correspondent transpired. And this is the manner in which it happened. Young Simpson, the postmaster, to whom Mrs. Houston had so imprudently given a portion of her confidence, found his curiosity piqued to discover who this forbidden correspondent might be, and after weeks of patient waiting, convinced himself that the letters addressed in a fair Italian hand to a certain person were those dropped into the box by Miss Helmstedt’s messenger, old Forrest. A few more observations confirmed this conviction. Then wishing to gain consequence in the eyes of Mrs. Houston, he availed himself of the first opportunity presented by the presence of that lady at the office to inform her of the discovery he had made.

“You are sure that is the name?” inquired the lady, in surprise.

“Yes, madam, that is the name, in a regular slanting hand. I always find a letter bearing that name in the box the moment after that old man has been seen about here, and never at any other time.”

“Very well; I thank you for your information; but mind! pray do not speak of this matter to any one but myself; for I would not like to have this subject discussed in town,” said Mrs. Houston.

“Oh, certainly not, madam! You may rely on me,” replied the young man, who, in half an hour afterward, laughed over the whole affair with a companion, both making very merry over the idea that the wealthy heiress, Miss Helmstedt, should be engaged to one lover and in private correspondence with another.

And so the ball set in motion by Nellie’s indiscretion rolled finely, never wanting a helping hand to propel it on its course; and gathered

as it rolled. The rumor changed its form: the gossip became slander And every one in the county, with the exception of Miss Helmstedt and her friends, “knew” that young lady was in “secret” correspondence with a low, disreputable sailor, whose acquaintance she had formed in some inexplicable manner, and the discovery of whose surreptitious visits to the island had been the proximate cause of her mother’s death.

Could Mrs. Houston have imagined half the evil that must accrue from her own imprudent conversation, she would have been touched with compunction; as it was, hearing nothing whatever of this injurious calumny, the guilty reveled in the rewards of “an approving conscience.” She kept her discovery of the mysterious name to herself; hinting to no one, least of all to Margaret, the extent of her knowledge upon this subject. And in order to throw the girl off her guard, she was careful never to resume the subject of the letters. And the plan succeeded so far that Margaret continued, at intervals of three or four weeks, to send off those mysterious letters, and thus the scandal grew and strengthened. That upon such slight grounds the good name of an innocent girl should have been assailed may astonish those unacquainted with the peculiar character of a neighborhood where the conduct of woman is governed by the most stringent conventionalism, and where such stringency is made necessary by the existing fact, that the slightest eccentricity of conduct, however innocent, or even meritorious it may be, is made the ground of the gravest animadversions.

Mrs. Houston, unconscious, as I said, of the rumors abroad, and biding her time for farther discoveries, treated Margaret with great kindness. Nellie had always, of all things, desired a daughter of her own. In her attached stepchild, Franky, she felt that she had quite a son of her own, and in Margaret she would have been pleased to possess the coveted daughter. As well as her capricious temper would allow her to do so, she sought to conduct herself as a mother toward the orphan girl; at times overwhelming her with flippant caresses and puerile attentions, which she might have mistaken for “the sweet, small courtesies of life,” but which were very distasteful

and unwelcome to one of Margaret Helmstedt’s profound, earnest, impassioned soul, and mournful life experiences.

The malaria of slander that filled all the air without must necessarily at last penetrate the precincts of home.

One day, a miserable, dark, drizzling day, near the last of November, Mr. Wellworth presented himself at the Bluff, and requested to see Mrs. Houston alone.

Nellie obeyed the summons, and went to receive the pastoral call in the front parlor across the hall from Margaret’s wing.

On entering the room she was struck at once by the unusually grave and even troubled look of the minister.

He arose and greeted her, handed a chair, and when she was seated resumed his own.

And then, after a little conversation, opened the subject of his visit.

“Mrs. Houston it is my very painful duty to advise you of the existence of certain rumors in regard to your amiable ward that I know to be as false as they are injurious, but with which I am equally certain you should be made acquainted.”

Nellie was really amazed—so unconscious was she of the effect of her own mischief-making. She drew out her perfumed pocket handkerchief to have it ready, and then inquired:

“To what purpose should I be informed of false, injurious rumors, sir? I know nothing of the rumors to which you refer.”

“I verily believe you, madam. But you should be made acquainted with them, as, in the event of their having been occasioned by any little act of thoughtlessness on the part of Miss Helmstedt, you may counsel that young lady and put a stop to this gossiping.”

“I do entreat you, sir, to speak plainly.”

“You must pardon me then, madam, if I take you at your word. It is currently reported, then, that Miss Helmstedt is in secret correspondence, ‘secret’ no longer, with a person of low and disreputable character, a waterman, skipper, or something of the

sort, whose acquaintance she formed in her mother’s lifetime and during her father’s absence, while she lived almost alone, on her native island. Now, of course, I know this rumor to be essentially false and calumnious; but I know also how delicate is the bloom on a young girl’s fair name, and how easily a careless handling will smirch it. Some thoughtless, perhaps some praiseworthy act on the part of this young creature—such as the sending of charitable donations through the post office, or something of the sort—may have given rise to this rumor, which should at once be met and put down by her friends. But I advise you, my dear madam, to speak to Miss Helmstedt and ascertain what ground, if any, however slight, there may be for this injurious rumor.”

For all answer, Mrs. Houston put her handkerchief to her face and began to weep.

“No, no, my dear Mrs. Houston, don’t take this too much to heart! these things must be firmly confronted and dealt with—not wept over.”

“Oh, sir! good sir! you don’t know! you don’t know! It is too true! Margaret gives me a world of anxiety.”

“Madam! you shock me! What is it you say?”

“Oh! sir, I am glad you came this morning! I have been wanting to ask your advice for a long time; but I did not like to. It is too true! Margaret is very imprudent!”

“Dear Heaven, madam! do you tell me that you knew of this report, and that it is not unfounded?”

“Oh! no, sir, I knew nothing of the report, as I told you before! I knew that Margaret was very, very imprudent, and gave me excessive uneasiness, but I did not dream that she had compromised herself to such an extent! Oh, never!” exclaimed Nellie, still and always unsuspicious of her own great share in creating the evil.

“You said that you had thought of asking my counsel. If you please to explain, my dear Mrs. Houston, you shall have the benefit of the best counsel my poor ability will furnish.”

“Oh! Heavens, sir! girls are not what they used to be when I was young—though I am scarcely middle-aged now—but they are not.”

“And Miss Helmstedt?”

“Oh, sir! Margaret is indeed in correspondence with some unknown man, whose very name I never heard in all my life before! She does all she can to keep the affair secret, and she thinks she keeps it so; but poor thing, having very little art, she cannot succeed in concealing the fact that she sends off these mysterious letters about once a month.”

“And do you not expostulate with her?” inquired the deeply-shocked minister.

“Oh, I did at first, sir, but I made no more impression upon her than if she had been a marble statue of Firmness. She would not tell me who her correspondent was, where he was, what he was, what was the nature of the acquaintance between them; in short, she would tell me nothing about him.”

“And can neither Colonel nor Mrs. Compton, nor your husband, impress her with the impropriety of this proceeding?”

“Oh, sir, they know nothing about it. No one in this house knows anything about Margaret’s conduct but myself. And the rumor you have just brought me has never reached them, I am sure.”

“Suppose you let me talk with my young friend. She means well, I am sure.”

“Well, sir, you shall have the opportunity you desire. But—excuse me for quoting for your benefit a homely adage—‘Trot sire, trot dam, and the colt will never pace!’ Margaret Helmstedt takes stubbornness from both parents, and may be supposed to have a double allowance,” said Mrs. Houston, putting her hand to the bell cord.

A servant appeared.

“Let Miss Helmstedt know that Mr. Wellworth desires to see her,” said Mrs. Houston.

The messenger withdrew, and soon returned with the answer that Miss Helmstedt would be glad to receive Mr. Wellworth in her own sitting-room.

“Will you accompany me hither then, Mrs. Houston?”

“No, I think not, sir. I fancy Miss Helmstedt prefers a private interview with her pastor. And I believe also that such a one would afford the best opportunity for your counseling Margaret.”

“Then you will excuse me, madam?”

“Certainly; and await here the issue of your visit,” said Mrs. Houston.

With a bow, the clergyman left the room, crossed the hall, and rapped at the door of Miss Helmstedt’s parlor.

It was opened by Hildreth, who stood in her starched puritanical costume, curtseying while the pastor entered the pretty boudoir. Margaret, still clothed in deep mourning, with her black hair plainly banded each side of her pale, clear, thoughtful face, sat in her low sewing-chair, engaged in plain needlework. She quietly laid it aside, and, with a warm smile of welcome, arose to meet her minister.

“You are looking better than when I saw you last, my child,” said the good pastor, pressing her hand, and mistaking the transient glow of pleasure for the permanent bloom of health.

“I am quite well, thank you, dear Mr. Wellworth! and you?”

“Always well, my child, thank Heaven.”

“And dearest Grace? I have not seen her so long.”

“Ah! she has even too good health, if possible! it makes her wild. We have to keep her at home to tame her.”

“But see—I am housekeeping here to myself, almost. My dear father has placed my maintenance upon the most lavish footing, and Mrs. Houston has given to his requests in regard to me the most liberal interpretation. See! I have, like a little princess, an establishment of my own. This wing of the house, a maid and messenger, a boat and horse; and my dear father has even written to have the carriage

brought from the island for my use, so that I may be able to visit or send for my friends at pleasure,” said Margaret, with a transient feeling of girlish delight in her independence.

“Yes, my child, I see; and I know that, in addition to this, you have an ample income. These are all great and unusual privileges for a young girl like yourself, not past childhood,” said Mr. Wellworth, very gravely.

“Oh! I know they are. I know, too, that these favors are lavished upon me in compassion for—to console me for—as if anything could make me cease to regret——” Here faltering, and finding herself on the verge of tears, Margaret paused, made an effort, controlled herself and resumed: “It is done in kindness toward her child; and I accept it all in the same spirit.”

“It is accorded in consideration of your grave and important position, my dear girl—do you never think of it? Young as you are, you are the affianced wife of the heir of this house.”

Again a transient flush of bashful joy chased the melancholy from Margaret’s face. Blushing, she dropped her eyes and remained silent.

“You think sometimes of your position, Margaret?” asked the clergyman, who, for his purpose, wished to lead and fix her mind upon this subject—“you remember sometimes that you are Ralph Houston’s promised wife?”

For an instant she lifted her dark eyelashes, darting one swift, shy, but most eloquent glance deep into his face, then, dropping them, crimsoned even to the edges of her black hair, and still continued silent.

“Ah! I see you do. I see you do. But do you know my dear, that something of the same discreet exclusiveness, reserve, circumspection, is demanded of a betrothed maiden as of a wife?” inquired the clergyman, solemnly.

Again her beautiful dark eyes were raised, in that quick, and quicklywithdrawn, penetrating, earnest, fervid, impassioned glance, that said, more eloquently than words would have spoken, “All that you

demand for him, and more, a millionfold, will my own heart, daily, hourly yield!” and then the blush deepened on her cheek, and she remained dumb.

“She, the promised wife, I mean, must not hold free conversation with gentlemen who are not her own near relatives; she must not correspond with them—she must not, in a word, do many things, which, though they might be perfectly innocent in a disengaged woman, would be very reprehensible in a betrothed maiden.”

Margaret’s color visibly fluctuated—her bosom perceptibly fluttered.

“Well, Margaret, what do you think of that which I have been telling you?”

“Oh! I know—I know you speak truly. I hope I know my duty and love to do it,” she said, in an agitated, confused manner; “but let us talk of something else, dear Mr Wellworth. Let us talk of my little, independent establishment here. When I spoke of the pleasant nature of my surroundings, it was to win your consent that dear Grace might come and be my guest for a week. She would be such a sweet comfort to me, and I could make her so happy here! If you will consent, I will send Forrest with the carriage for her to-morrow. Say, will you, dear Mr. Wellworth?”

“Perhaps; we will talk about that by and by. Margaret,” he said, suddenly lowering his voice, “dismiss your woman, I wish to speak alone with you, my child.”

“Hildreth, go, but remain in sound of my bell,” said Miss Helmstedt.

As soon as Hildreth had left the room, Mr Wellworth drew his chair beside the low seat of Margaret, took her hand, and would have held it while he spoke, but that she, who always shrank even from the fatherly familiarity of her pastor, very gently withdrew it, and respectfully inquired:

“What was it you wished to say to me, dear Mr. Wellworth?”

“A very serious matter, my dear child. Margaret, I have no art in circumnavigating a subject. I have been trying to approach gradually the subject of my visit to you this morning, and I have not

succeeded. I am no nearer than when I first entered. I know not how to ‘break’ bad news——”

“In a word, sir, has misfortune happened to any of my friends?” inquired Margaret, with a pale cheek, but with a strange, calm voice.

“No; that were more easily told than what I have to tell,” said the minister, solemnly.

“Please go on then, sir, and let me know the worst at once.”

“Then, my dear Margaret, I have been informed that you, a betrothed wife, have an intimate male correspondent, who is neither your father nor your affianced husband, and whose name and character, and relations with yourself, you decline to divulge?”

Margaret grew ashen pale, clasped her hands, compressed her lips, and remained silent.

“What have you to say to this charge, Margaret?”

There was a pause, while Mr. Wellworth gazed upon the maiden’s steadfast, thoughtful face. She reasoned with herself; she struggled with herself. It occurred to her to say, “My correspondent is a grayhaired man, whom I have never set eyes upon.” But immediately, she reflected. “No, this may put suspicion upon the true scent; I must say nothing.”

“Well, Margaret, what have you to answer to this charge?”

“Nothing, sir.”

“Nothing?”

“Nothing.”

“You admit it, then?”

“I neither admit nor deny it!”

“Margaret, this will never do. Are you aware that you seriously imperil, nay, more, that you gravely compromise your good name?”

Her pale cheek grew paler than before, the tightly-clasped fingers trembled, the compressed lips sprang quivering apart, and then

closed more firmly than ever It had occurred to her to say: “But this correspondence is solely a business affair, with one of whom I have no personal knowledge whatever.” But then came the reflection: “If I give them this explanation, this ever so slight clue, these worldlywise people will follow it up until they unravel the whole mystery, and I shall have proved myself a cowardly traitor to her confidence. No, I must be dumb before my accusers!”

“You do not speak, Margaret.”

“I have nothing to say, sir!”

“Ah, dear Heaven! I see that I must not ‘prophesy smooth things’ to you, my girl. I must not spare the truth! Listen, then, Miss Helmstedt: Your name has become a byword in the village shops! What now will you do?”

It was on her pallid lips to say: “I will trust in God;” but she said it only in her heart, adding: “I must not even insist upon my innocence; for if they believe me, they will be forced to find the right track to this scent.”

“Margaret Helmstedt, why do you not answer me?”

“Because, sir, I have nothing to say.”

“Nothing to say?”

“Nothing—nothing to say!”

“Listen to me, then. You seem to have some regard for your betrothed husband. You seem even to understand the duty you owe him! Think, I beg you, what must be the feelings of a proud and honorable man like Ralph Houston, on returning to this neighborhood and finding the name and fame of his affianced bride lightly canvassed?”

It was piteous to see how dark with woe her face became. Her hands were clenched until it seemed as though the blood must start from her finger nails; but not one word escaped her painfully-compressed lips.

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